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The theory of second-harmonic generation (SHG) that is due to quadrupole and magnetic-dipole second-order optical susceptibilities is developed for monochromatic, focused beams of arbitrary transverse mode structure and polarization character. The strength of SHG depends sensitively on the polarization character of the beam. © 1981 Optical Society of America.
Bryan D. McCloskey, D.S. Bethune, et al.
Journal of Physical Chemistry Letters
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